Improved oxidation properties from a reduced B content in sputter-deposited TiBx thin films

نویسندگان

چکیده

Transition-metal diboride thin films, which have high melting points, excellent hardness, and good chemical thermal conductivity, severely suffer from rapid oxidation in air. Here, we explore the influence of varying B content resulting nanostructure change on properties TiBx with x = 1.43, 2.20, 2.70. Results show that all as-deposited layers columnar structure. The column boundaries TiB2.20 TiB2.70 films grown by direct current magnetron sputtering (DCMS) are B-rich, while TiB1.43 high-power impulse (HiPIMS) no apparent grain boundary phases contain Ti-rich planar defects. rate air-annealed at 400 °C up to 48 h is significantly lower than films. TiB1.43, TiB2.20, was measured 2.9 ± 1.5, 7.1 1.0, 20.0 5.0 nm/h, respectively, spallation even as thick oxide scales 0.5 μm any improved resistance can be explained absence B-rich tissue phase understoichiometric a interlaces nanocolumnar TiB2 structures corresponding overstoichiometric An easy pathway thus eliminated.

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ژورنال

عنوان ژورنال: Surface & Coatings Technology

سال: 2021

ISSN: ['1879-3347', '0257-8972']

DOI: https://doi.org/10.1016/j.surfcoat.2021.127353